I think they do Not look toddlerish ,but they Do look a bit mixed message stylistically at least with some of the looks.
The Danskos look like the Chucks as mentioned previously. As such they read Sporty and/or Rocker Chic . So color blocking,athletic vibe pieces work beautifully with them.
Some of the outfits pictured have a more Bohemian or Feminine Romantic look ( blue Ikat print shirt, floppy sun hat , soft feminine beige sweater) so in picture 1. the top half is boho/ fem and the bottom sporty rocker.
My solution? You NEED a pair of boho / feminine shoes ( Oh ! The TRAGEDY! A woman being told she has to get MORE Shoes! ) I'd suggest since you like and can successfully wear chunky shoes ,getting a Birkenstock or lookalike to wear with the boho looks. Or a sandal from Softwalk,Walking Cradles,b.o.c.,Born etc.